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A detailed understanding of the combustion mechanisms is required for optimizing the complex relationship between fuel economy, combustion emissions, and performance; this is dependent on the accurate diagnosis of the combustion system with up-todate new measurement techniques. It is not inappropriate to describe the history of combustion research as the history of combustion diagnostics. Recently, laser-based nonintrusive diagnostic techniques, due to their many advantages that conventional probes do not possess, have been finding an explosive application in the field of combustion research, which can provide new phenomenological insight into the fundamental behavior of the combustion system.